Another nice place, that appeared in 007's Goldfinger, the Hotel Belvedere. Much more rustic, but an adventure in itself:
Belvédère am Rhonegletscher - Seit 130 Jahren CH-3999 Belvédère am Furkapass Wallis/Schweiz, 2‘300 m.ü.M.
After that you cross over the Furka to Andermatt, then down north to Luzern.
Again, no matter where you go, if you are in the Alps, you can not go wrong.